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Antibodies Against Specific MUC16 Glycosylation Sites Inhibit Ovarian Cancer Growth

ACS Chem Biol. 2017 Aug 18;12(8):2085-2096. doi: 10.1021/acschembio.7b00305. Epub 2017 Jun 28.

Abstract

Expression of the retained C-terminal extracellular portion of the ovarian cancer glycoprotein MUC16 induces transformation and tumor growth. However, the mechanisms of MUC16 oncogenesis related to glycosylation are not clearly defined. We establish that MUC16 oncogenic effects are mediated through MGAT5-dependent N-glycosylation of two specific asparagine sites within its 58 amino acid ectodomain. Oncogenic signaling from the C-terminal portion of MUC16 requires the presence of Galectin-3 and growth factor receptors colocalized on lipid rafts. These effects are blocked upon loss of either Galectin-3 expression or activity MGAT5. Using synthetic MUC16 glycopeptides, we developed novel N-glycosylation site directed monoclonal antibodies that block Galectin-3-mediated MUC16 interactions with cell surface signaling molecules. These antibodies inhibit invasion of ovarian cancer cells, directly blocking the in vivo growth of MUC16-bearing ovarian cancer xenografts, elucidating new therapeutic modalities.

MeSH terms

  • Animals
  • Antibodies, Monoclonal / pharmacology*
  • Binding Sites
  • CA-125 Antigen / chemistry*
  • CA-125 Antigen / genetics
  • CA-125 Antigen / metabolism
  • Carcinogenesis / drug effects*
  • Cell Line, Tumor
  • Cell Proliferation / drug effects
  • ErbB Receptors / metabolism
  • Female
  • Gene Expression Regulation, Neoplastic / drug effects
  • Glycosylation / drug effects
  • Humans
  • Membrane Proteins / chemistry*
  • Membrane Proteins / genetics
  • Membrane Proteins / metabolism
  • Mice
  • Ovarian Neoplasms / physiopathology
  • Signal Transduction

Substances

  • Antibodies, Monoclonal
  • CA-125 Antigen
  • MUC16 protein, human
  • Membrane Proteins
  • EGFR protein, human
  • ErbB Receptors