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The eruption of both the Eyjafjallajokull (April 2010) and Grimsvotn (May 2011) volcanoes cumulated with two moments that gave headaches to the authorities and air traffic, and their impact on the environment upon Iasi region have been studied by means of different tools evidencing the complexity of the phenomena. In order to evidence the intrusion of pollutants in the cloud systems and to obtain additional data on the intrusion when the ash cloud was over our country, LIDAR measurements, meteorological (NMA), Satellite data (EUMETSAT), and various forecasting models (ECMWF, VAAC-Met Office, HYSPLIT) have been used. The new 3D Atmospheric Observatory Site of the Alexandru Ioan Cuza University of Iasi, as part of RADO (Romanian Atmospheric 3D Observatory) is presented, too.