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Interfacial Engineering for Oriented Crystal Growth toward Dendrite-Free Zn Anode for Aqueous Zinc Metal Battery.

Author information

Affiliations

  • 1. Frontiers Science Center for New Organic Matter, Key Laboratory of Advanced Energy Materials Chemistry (Ministry of Education), Renewable Energy Conversion and Storage Center (RECAST), College of Chemistry, Nankai University, Tianjin, 300071, China.
      Authors
    • Zhou X 1, 2
    • Wen B 1
    • Cai Y 1
    • Zhao Q 1
    • Li F 1
    (5 authors)
  • 2. Institute for Carbon Neutralization, College of Chemistry and Materials Engineering, Wenzhou University, Wenzhou, Zhejiang, 325035, China.
      Authors
    • Zhou X 1, 2
    • Chen X 2
    • Li L 2
    • Chou SL 2
    (4 authors)

ORCIDs linked to this article

Angewandte Chemie (International ed. in English), 11 Apr 2024, 63(21):e202402342
https://doi.org/10.1002/anie.202402342 PMID: 38491787 

Abstract 

Zn deposition with a surface-preferred (002) crystal plane has attracted extensive attention due to its inhibited dendrite growth and side reactions. However, the nucleation and growth of the Zn(002) crystal plane are closely related to the interfacial properties. Herein, oriented growth of Zn(002) crystal plane is realized on Ag-modified surface that is directly visualized by in situ atomic force microscopy. A solid solution HCP-Zn (~1.10 at. % solubility of Ag, 30 °C) is formed on the Ag coated Zn foil (Zn@Ag) and possesses the same crystal structure as Zn to reduce its nucleation barrier caused by their lattice mismatch. It merits oriented Zn deposition and corrosion-resistant surface, and presents long cycling stability in symmetric cells and full cells coupled with V2O5 cathode. This work provides insights into interfacial regulation of Zn anodes for high-performance aqueous zinc metal batteries.

Full text links 

Read article at publisher's site: https://doi.org/10.1002/anie.202402342

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Funding 

Funders who supported this work.

China Postdoctoral Science Foundation (1)

National Natural Science Foundation of China (4)