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Enhanced mineralization of Reactive Black 5 by waste iron oxide via photo-Fenton process

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Abstract

Advanced oxidation process is a promising technology for the treatment of azo dye wastewater, owing to its high degradation performance and less secondary contamination. Herein, the mineralization of azo dye Reactive Black 5 (RB5) by the heterogeneous photo-Fenton process was investigated in a three-phase fluidized bed reactor. The waste iron oxide (denoted as BT) obtained from tannery wastewater process with Fenton’s reagent was selected as a heterogeneous catalyst. The introduction of BT to the UV/H2O2 process (UV/H2O2/BT) shows obviously higher mineralization efficiency because ferric complexes of carboxylic acid, the degradation intermediates of RB5, could be readily decomposed by UV irradiation. The decolorization was achieved by homogenous photo-Fenton reaction induced by leached iron, while the mineralization was contributed to heterogeneous oxidation. Under the conditions of 254 nm UV irradiation, 19.00 mM H2O2, 2.0 g L–1 catalyst loading and natural pH0 of 5.0, 90.2% TOC removal of RB5 could be achieved. The catalyst indicated an acceptable stability and reusability after four cycles. The proposed heterogeneous photo-Fenton process with stable performance is environmental-friendly for the mineralization of RB5.

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Authors and Affiliations

  1. Department of Environmental Science and Engineering, Wuhan University, Wuhan, 430079, China

    Weihua Tan, Jia Ai, Yuanrou Fan, Xiang Liu, Yuncheng Xu & Hui Zhang

  2. Department of Chemical Engineering, National Cheng-Kung University, Tainan, 70101, Taiwan

    Jia Ai & Yao-Hui Huang

  3. Sustainable Environmental Research Center, National Cheng-Kung University, Tainan, 70101, Taiwan

    Yao-Hui Huang

Authors
  1. Weihua Tan
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  2. Jia Ai
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  3. Yuanrou Fan
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  4. Xiang Liu
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  5. Yuncheng Xu
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  6. Hui Zhang
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  7. Yao-Hui Huang
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Correspondence to Hui Zhang or Yao-Hui Huang.

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Tan, W., Ai, J., Fan, Y. et al. Enhanced mineralization of Reactive Black 5 by waste iron oxide via photo-Fenton process. Res Chem Intermed 46, 4423–4431 (2020). https://doi.org/10.1007/s11164-020-04212-w

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  • DOI: https://doi.org/10.1007/s11164-020-04212-w

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