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Design of selectively activated anticancer prodrugs: elimination and cyclization strategies

Curr Med Chem Anticancer Agents. 2002 Mar;2(2):155-85. doi: 10.2174/1568011023354173.

Abstract

Cancer chemotherapy is associated with severe side effects which may be reduced by selective liberation, at the tumour site, of a cytotoxic agent from a non-toxic prodrug. Several strategies are used to achieve the required selective activation: with enzymes which are present in higher concentration in, or close, to the tumour (beta-glucuronidase, plasmin), with enzymes covalently linked to a macromolecular carrier able to recognize antigen positive cancer cells (ADEPT: Antibody Directed Enzyme Prodrug Therapy) or with reductive processes which are favoured in an hypoxic environment. Most of the prodrugs include a linker (or spacer) between the trigger and the drug (or effector). The design of such linkers is crucial in order to achieve a fast drug liberation under physiological conditions. The linker groups may be classified in two categories based on elimination or cyclization processes. The advantages and the limitations of each strategy are discussed.

Publication types

  • Research Support, Non-U.S. Gov't
  • Review

MeSH terms

  • Animals
  • Antineoplastic Agents / chemical synthesis*
  • Antineoplastic Agents / pharmacology
  • Cross-Linking Reagents
  • Cyclization
  • Humans
  • Prodrugs / chemical synthesis*
  • Prodrugs / pharmacology
  • Structure-Activity Relationship

Substances

  • Antineoplastic Agents
  • Cross-Linking Reagents
  • Prodrugs