Nothing Special   »   [go: up one dir, main page]

Skip to main content

Thank you for visiting nature.com. You are using a browser version with limited support for CSS. To obtain the best experience, we recommend you use a more up to date browser (or turn off compatibility mode in Internet Explorer). In the meantime, to ensure continued support, we are displaying the site without styles and JavaScript.

  • Article
  • Published:

Theory of universal incoherent metallic transport

Abstract

The anomalous transport of important materials such as high-temperature superconductors and other ‘bad metals’ is not well understood theoretically. In an incoherent metal, transport is controlled by the collective diffusion of energy and charge rather than by quasiparticle or momentum relaxation. Here, we explore the possibility of a universal bound D νF2/(kBT) on the underlying diffusion constants in an incoherent metal. Such a bound is loosely motivated by results from holographic duality, the uncertainty principle and measurements of diffusion in strongly interacting non-metallic systems. Metals close to saturating this bound are shown to have a linear-in-temperature resistivity with an underlying dissipative timescale matching that recently deduced from experimental data on a wide range of metals. This bound may therefore be responsible for the ubiquitous appearance of high-temperature regimes in metals with T-linear resistivity. To establish this calls for direct measurements of diffusive processes and of charge susceptibilities in incoherent metals.

This is a preview of subscription content, access via your institution

Access options

Buy this article

Prices may be subject to local taxes which are calculated during checkout

Figure 1: Quasiparticle bounds versus incoherent bounds.
Figure 2: Lorenz ratio as a function of temperature.

Similar content being viewed by others

References

  1. Bruin, J. A. N., Sakai, H., Perry, R. S. & Mackenzie, A. P. Similarity of scattering rates in metals showing T-linear resistivity. Science 339, 804–807 (2013).

    Article  ADS  Google Scholar 

  2. Sachdev, S. Quantum Phase Transitions (CUP, 1999).

    MATH  Google Scholar 

  3. Zaanen, J. Superconductivity: Why the temperature is high. Nature 430, 512–513 (2004).

    Article  ADS  Google Scholar 

  4. Hussey, N. E., Takenaka, K. & Takagi, H. Universality of the Mott–Ioffe–Regel limit in metals. Phil. Mag. 84, 2847–2864 (2004).

    Article  ADS  Google Scholar 

  5. Gunnarsson, O., Calandra, M. & Han, J. E. Colloquium: Saturation of electrical resistivity. Rev. Mod. Phys. 75, 1085–1099 (2003).

    Article  ADS  Google Scholar 

  6. Emery, V. J. & Kivelson, S. A. Superconductivity in bad metals. Phys. Rev. Lett. 74, 3253–3256 (1995).

    Article  ADS  Google Scholar 

  7. Policastro, G., Son, D. T. & Starinets, A. O. The shear viscosity of strongly coupled N = 4 supersymmetric Yang-Mills plasma. Phys. Rev. Lett. 87, 081601 (2001).

    Article  ADS  Google Scholar 

  8. Herzog, C. P., Kovtun, P., Sachdev, S. & Son, D. T. Quantum critical transport, duality, and M-theory. Phys. Rev. D 75, 085020 (2007).

    Article  ADS  MathSciNet  Google Scholar 

  9. Hartnoll, S. A., Kovtun, P. K., Muller, M. & Sachdev, S. Theory of the Nernst effect near quantum phase transitions in condensed matter, and in dyonic black holes. Phys. Rev. B 76, 144502 (2007).

    Article  ADS  Google Scholar 

  10. Kovtun, P., Son, D. T. & Starinets, A. O. Viscosity in strongly interacting quantum field theories from black hole physics. Phys. Rev. Lett. 94, 111601 (2005).

    Article  ADS  Google Scholar 

  11. Son, D. T. & Starinets, A. O. Viscosity, black holes, and quantum field theory. Annu. Rev. Nucl. Part. Sci. 57, 95–118 (2007).

    Article  ADS  Google Scholar 

  12. Cremonini, S. The shear viscosity to entropy ratio: A status report. Mod. Phys. Lett. B 25, 1867–1888 (2011).

    Article  ADS  MathSciNet  MATH  Google Scholar 

  13. Adams, A., Carr, L. D., Schäfer, T., Steinberg, P. & Thomas, J. E. Strongly correlated quantum fluids: Ultracold quantum gases, quantum chromodynamic plasmas, and holographic duality. New J. Phys. 14, 115009 (2012).

    Article  ADS  MathSciNet  Google Scholar 

  14. Ziman, J. M. Electrons and Phonons (OUP, 1960).

    MATH  Google Scholar 

  15. Forster, D. Hydrodynamic Fluctuations, Broken Symmetry, and Correlation Functions (W. A. Benjamin, Advanced Book Classics, 1975).

    Google Scholar 

  16. Hartnoll, S. A. & Hofman, D. M. Locally critical resistivities from umklapp scattering. Phys. Rev. Lett. 108, 241601 (2012).

    Article  ADS  Google Scholar 

  17. Mahajan, R., Barkeshli, M. & Hartnoll, S. A. Non-Fermi liquids and the Wiedemann–Franz law. Phys. Rev. B 88, 125107 (2013).

    Article  ADS  Google Scholar 

  18. Jung, P. & Rosch, A. Lower bounds for the conductivities of correlated quantum systems. Phys. Rev. B 75, 245104 (2007).

    Article  ADS  Google Scholar 

  19. Hartnoll, S. A. & Herzog, C. P. Impure AdS/CFT correspondence. Phys. Rev. D 77, 106009 (2008).

    Article  ADS  MathSciNet  Google Scholar 

  20. Basov, D. N., Averitt, R. D., van der Marel, D., Dressel, M. & Haule, K. Electrodynamics of correlated electron materials. Rev. Mod. Phys. 83, 471–541 (2011).

    Article  ADS  Google Scholar 

  21. Fisher, M. P. A., Weichman, P. B., Grinstein, G. & Fisher, D. S. Boson localization and the superfluid-insulator transition. Phys. Rev. B 40, 546–570 (1989).

    Article  ADS  Google Scholar 

  22. Witczak-Krempa, W., Ghaemi, P., Senthil, T. & Kim, Y. B. Universal transport near a quantum critical Mott transition in two dimensions. Phys. Rev. B 86, 245102 (2012).

    Article  ADS  Google Scholar 

  23. Metlitski, M. A. & Sachdev, S. Quantum phase transitions of metals in two spatial dimensions: II. Spin density wave order. Phys. Rev. B 82, 075128 (2010).

    Article  ADS  Google Scholar 

  24. Prange, R. E. & Kadanoff, L. P. Transport theory for electron–phonon interactions in metals. Phys. Rev. 134, A566 (1964).

    Article  ADS  MATH  Google Scholar 

  25. Koschorreck, M., Pertot, D., Vogt, E. & Köhl, M. Universal spin dynamics in two-dimensional Fermi gases. Nature Phys. 9, 405–409 (2013).

    Article  ADS  Google Scholar 

  26. Spivak, B. & Kivelson, S. A. Transport in two dimensional electronic micro-emulsions. Ann. Phys. 321, 2071–2115 (2006).

    Article  ADS  MATH  Google Scholar 

  27. Andreev, A. V., Kivelson, S. A. & Spivak, B. Hydrodynamic description of transport in strongly correlated electron systems. Phys. Rev. Lett. 106, 256804 (2011).

    Article  ADS  Google Scholar 

  28. Balasubramanian, K. & Herzog, C. P. Losing forward momentum holographically. Class. Quantum Gravity 31, 125010 (2014).

    Article  ADS  MATH  Google Scholar 

  29. Davison, R. A., Schalm, K. & Zaanen, J. Holographic duality and the resistivity of strange metals. Phys. Rev. B 89, 245116 (2014).

    Article  ADS  Google Scholar 

  30. Georges, A., Kotliar, G., Krauth, W. & Rozenberg, M. J. Dynamical mean-field theory of strongly correlated fermion systems and the limit of infinite dimensions. Rev. Mod. Phys. 68, 13–125 (1996).

    Article  ADS  MathSciNet  Google Scholar 

  31. Deng, X. et al. How bad metals turn good: Spectroscopic signatures of resilient quasiparticles. Phys. Rev. Lett. 110, 086401 (2013).

    Article  ADS  Google Scholar 

  32. Pálsson, G. & Kotliar, G. Thermoelectric response near the density driven Mott transition. Phys. Rev. Lett. 80, 4775 (1998).

    Article  ADS  Google Scholar 

  33. Kovtun, P. & Ritz, A. Universal conductivity and central charges. Phys. Rev. D 78, 066009 (2008).

    Article  ADS  Google Scholar 

  34. Imada, M., Fujimori, A. & Tokura, Y. Metal-insulator transitions. Rev. Mod. Phys. 70, 1039–1263 (1998).

    Article  ADS  Google Scholar 

  35. Takenaka, K., Nohara, J., Shiozaki, R. & Sugai, S. Incoherent charge dynamics of La2−xSrxCuO4: Dynamical localization and resistivity saturation. Phys. Rev. B 68, 134501 (2003).

    Article  ADS  Google Scholar 

  36. Van der Marel, D. et al. Quantum critical behaviour in a high-Tc superconductor. Nature 425, 271–274 (2003).

    Article  ADS  Google Scholar 

  37. Hwang, J., Timusk, T. & Gu, G. D. Doping dependent optical properties of Bi2Sr2CaCu2O8+δ . J. Phys. Condens. Matter 19, 125208 (2007).

    Article  ADS  Google Scholar 

  38. Boris, A. V. et al. In-plane spectral weight shift of charge carriers in YBa2Cu3O6.9 . Science 304, 708–710 (2004).

    Article  ADS  Google Scholar 

  39. Wu, D. et al. Effects of magnetic ordering on dynamical conductivity: Optical investigations of EuFe2As2 single crystals. Phys. Rev. B 79, 155103 (2009).

    Article  ADS  Google Scholar 

  40. Schafgans, A. A. et al. Electronic correlations and unconventional spectral weight transfer in the high-temperature pnictide BaFe2−xCoxAs2 superconductor using infrared spectroscopy. Phys. Rev. Lett. 108, 147002 (2012).

    Article  ADS  Google Scholar 

  41. Takenaka, K. et al. Collapse of coherent quasiparticle states in θ-(BEDT–TTF)2I3 observed by optical spectroscopy. Phys. Rev. Lett. 95, 227801 (2005).

    Article  ADS  Google Scholar 

  42. Jönsson, P. E. et al. Correlation-driven heavy-fermion formation in LiV2O4 . Phys. Rev. Lett. 99, 167402 (2007).

    Article  ADS  Google Scholar 

  43. Wang, N. L. et al. Infrared probe of the electronic structure and charge dynamics of Na0.7CoO2 . Phys. Rev. Lett. 93, 237007 (2004).

    Article  ADS  Google Scholar 

  44. Lee, Y. S. et al. Non-Fermi liquid behavior and scaling of the low-frequency suppression in the optical conductivity spectra of CaRuO3 . Phys. Rev. B 66, 041104(R) (2002).

    Article  ADS  Google Scholar 

  45. Witczak-Krempa, W. & Sachdev, S. The quasi-normal modes of quantum criticality. Phys. Rev. B 86, 235115 (2012).

    Article  ADS  Google Scholar 

  46. Deng, X., Sternbach, A., Haule, K., Basov, D. N. & Kotliar, G. Shining light on transition metal oxides: Unveiling the hidden Fermi liquid. Preprint at http://arXiv.org/abs/1404.6480 (2014)

  47. Jaramillo, R., Ha, S. D., Silevitch, D. M. & Ramanathan, S. Origins of bad-metal conductivity and the insulator–metal transition in the rare-earth nickelates. Nature Phys. 10, 304–307 (2014).

    Article  ADS  Google Scholar 

  48. Ando, Y., Lavrov, A. N., Komiya, S., Segawa, K. & Sun, X. F. Mobility of the doped holes and the antiferromagnetic correlations in underdoped high-Tc cuprates. Phys. Rev. Lett. 87, 017001 (2001).

    Article  ADS  Google Scholar 

  49. Hussey, N. E. et al. Dichotomy in the T-linear resistivity in hole-doped cuprates. Phil. Trans. R. Soc. A 369, 1626–1639 (2011).

    Article  ADS  Google Scholar 

  50. Orenstein, J. et al. Frequency- and temperature-dependent conductivity in YBa2Cu3O6+x crystals. Phys. Rev. B 42, 6342–6362 (1990).

    Article  ADS  Google Scholar 

  51. Uchida, S. et al. Optical spectra of La2−xSrxCuO4: Effect of carrier doping on the electronic structure of the CuO2 plane. Phys. Rev. B 43, 7942–7954 (1991).

    Article  ADS  Google Scholar 

  52. Taillefer, L. Scattering and pairing in cuprate superconductors. Annu. Rev. Condens. Matter Phys. 1, 51–70 (2010).

    Article  ADS  Google Scholar 

  53. Tanatar, M. A., Paglione, J., Petrovic, C. & Taillefer, L. Anisotropic violation of the Wiedemann–Franz law at a quantum critical point. Science 316, 1320–1322 (2007).

    Article  ADS  Google Scholar 

  54. Pfau, H. et al. Thermal and electrical transport across a magnetic quantum critical point. Nature 484, 493–497 (2012).

    Article  ADS  Google Scholar 

  55. Zhang, Y. et al. Determining the Wiedemann–Franz ratio from the thermal Hall conductivity: Application to Cu and YBa2Cu3O6.95 . Phys. Rev. Lett. 84, 2219–2222 (2000).

    Article  ADS  Google Scholar 

  56. Wu, X. D. et al. Thermal diffusivity of Bi2Sr2CaCu2O8 single crystals. Physica C 218, 417–423 (1993).

    Article  ADS  Google Scholar 

  57. Wu, X. D., Kino, G. S., Fanton, J. T. & Kapitulnik, A. Photothermal microscope for high-Tc superconductors and charge density waves. Rev. Sci. Instrum. 64, 3321–3327 (1993).

    Article  ADS  Google Scholar 

  58. Weber, C. P. et al. Observation of spin Coulomb drag in a two-dimensional electron gas. Nature 437, 1330–1333 (2005).

    Article  ADS  Google Scholar 

  59. Gedik, N., Orenstein, J., Liang, R., Bonn, D. A. & Hardy, W. N. Diffusion of nonequilibrium quasi-particles in a cuprate superconductor. Science 300, 1410–1412 (2003).

    Article  ADS  Google Scholar 

  60. Donos, A. & Gauntlett, J. P. Novel metals and insulators from holography. JHEP 1406, 007 (2014).

    Article  ADS  Google Scholar 

  61. Goutéraux, B. Charge transport in holography with momentum dissipation. JHEP 1404, 181 (2014).

    Article  ADS  Google Scholar 

  62. Mukerjee, S., Oganesyan, V. & Huse, D. Towards a statistical theory of transport by strongly-interacting lattice fermions. Phys. Rev. B 73, 035113 (2006).

    Article  ADS  Google Scholar 

  63. Kadanoff, L. P. & Martin, P. C. Hydrodynamic equations and correlation functions. Ann. Phys. 24, 419–469 (1963).

    Article  ADS  MathSciNet  MATH  Google Scholar 

Download references

Acknowledgements

I have benefited greatly from discussions with A. Kapitulnik, G. Kotliar, B. Laughlin, A. Mackenzie, R. McKenzie, V. Oganesyan, J. Orenstein, B. Spivak and especially S. Kivelson. S.A.H. is partially financially supported by a DOE Early Career Award and by a Sloan fellowship.

Author information

Authors and Affiliations

Authors

Corresponding author

Correspondence to Sean A. Hartnoll.

Ethics declarations

Competing interests

The author declares no competing financial interests.

Rights and permissions

Reprints and permissions

About this article

Check for updates. Verify currency and authenticity via CrossMark

Cite this article

Hartnoll, S. Theory of universal incoherent metallic transport. Nature Phys 11, 54–61 (2015). https://doi.org/10.1038/nphys3174

Download citation

  • Received:

  • Accepted:

  • Published:

  • Issue Date:

  • DOI: https://doi.org/10.1038/nphys3174

This article is cited by

Search

Quick links

Nature Briefing

Sign up for the Nature Briefing newsletter — what matters in science, free to your inbox daily.

Get the most important science stories of the day, free in your inbox. Sign up for Nature Briefing